Online Exploring the Gaseous Oil Fumes from Oleic Acid Thermal Oxidation by Synchrotron Radiation Photoionization Mass Spectrometry

被引：2
|
作者：
Qian, Bing [1 ]
Hu, Yonghua [2 ]
Xu, Minggao [1 ]
Yang, Jiuzhong [1 ]
Liu, Chengyuan [1 ]
Pan, Yang [1 ]
机构：
[1] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China
[2] China Tobacco Anhui Ind Co Ltd, Ctr Technol, Hefei 230088, Anhui, Peoples R China
来源：
JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY | 2023年 / 34卷 / 12期
基金：
中国国家自然科学基金;
关键词：
oil fume; photoionization mass spectrometry; oleic acid thermal oxidation; online; synchrotronradiation; VOLATILE ORGANIC-COMPOUNDS; GAS-CHROMATOGRAPHY; LUNG-CANCER; TEMPERATURE OXIDATION; CARBONYL-COMPOUNDS; COOKING FUMES; EMISSIONS; PHASE; RISK; TIME;
D O I：
10.1021/jasms.3c00259
中图分类号：
Q5 [生物化学];
学科分类号：
071010 ; 081704 ;
摘要：
Cooking oil fumes are an intricate and dynamic mixture containing a variety of poisonous and hazardous substances, and their real-time study remains challenging. Based on tunable synchrotron radiation photoionization mass spectrometry (SR-PIMS), isomeric/isobaric compounds in the gaseous oil fumes from oleic acid thermal oxidation were determined in real time and distinguished by photoionization efficiency (PIE) curve simulation combined with multiple linear regression (MLR) analysis. A series of common carcinogens such as formaldehyde, acetaldehyde, acrolein, and several unreported chemicals including diethyl ether and formyl-cyclohexane were successfully characterized. Moreover, time-resolved profiles of certain components in gaseous oil fumes were monitored for 55 h. Distinct evolutionary processes were observed, indicating the consumption and formation of parent molecules, intermediates, and final products.
引用
收藏
页码：2680 / 2690
页数：11
相关论文
共 11 条
  • [1] Study on the thermal oxidation of oleic, linoleic and linolenic acids by synchrotron radiation photoionization mass spectrometry
    Qian, Bing
    Hu, Yonghua
    Xu, Minggao
    Yang, Jiuzhong
    Liu, Chengyuan
    Pan, Yang
    RAPID COMMUNICATIONS IN MASS SPECTROMETRY, 2023, 37 (21)
  • [2] Ion Dissociation of Hydrazoic Acid Investigated by Synchrotron-Radiation-Based Photoionization Mass Spectrometry
    Quinto-Hernandez, Alfredo
    Wodtke, Alec M.
    Lee, Yin-Yu
    Huang, Tzu-Ping
    Pan, Wan-Chun
    Lin, Jim Jr-Min
    JOURNAL OF PHYSICAL CHEMISTRY A, 2009, 113 (16): : 3822 - 3829
  • [3] Online Monitoring the Key Intermediates and Volatile Compounds Evolved from Green Tea Roasting by Synchrotron Radiation Photoionization Mass Spectrometry
    Qi, Keke
    Xu, Minggao
    Yin, Hao
    Wu, Liutian
    Hu, Yonghua
    Yang, Jiuzhong
    Liu, Chengyuan
    Pan, Yang
    JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY, 2021, 32 (06) : 1402 - 1411
  • [4] Online Analysis of Volatile Products from Bituminous Coal Pyrolysis with Synchrotron Vacuum Ultraviolet Photoionization Mass Spectrometry
    Jia, Liangyuan
    Weng, Junjie
    Wang, Yu
    Sun, Shaobo
    Zhou, Zhouyue
    Qi, Fei
    ENERGY & FUELS, 2013, 27 (02) : 694 - 701
  • [5] Benzene decomposition by non-thermal plasma: A detailed mechanism study by synchrotron radiation photoionization mass spectrometry and theoretical calculations
    Liang, Yuting
    Li, Jiayi
    Xue, Yingying
    Tan, Ting
    Jiang, Zhi
    He, Yaoyu
    Shangguan, Wenfeng
    Yang, Jiuzhong
    Pan, Yang
    JOURNAL OF HAZARDOUS MATERIALS, 2021, 420
  • [6] New Insights into Low-Temperature Oxidation of Propane from Synchrotron Photoionization Mass Spectrometry and Multiscale Informatics Modeling
    Welz, Oliver
    Burke, Michael P.
    Antonov, Ivan O.
    Goldsmith, C. Franklin
    Savee, John D.
    Osborn, David L.
    Taatjes, Craig A.
    Klippenstein, Stephen J.
    Sheps, Leonid
    JOURNAL OF PHYSICAL CHEMISTRY A, 2015, 119 (28): : 7116 - 7129
  • [7] Illustrating the Fate of Methyl Radical in Photocatalytic Methane Oxidation over Ag-ZnO by in situ Synchrotron Radiation Photoionization Mass Spectrometry
    Liu, Chengyuan
    Qian, Bing
    Xiao, Tianci
    Lv, Chunchun
    Luo, Jinsong
    Bao, Jun
    Pan, Yang
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2023, 62 (32)
  • [8] Free-radical triggered formation of dioxins from 2-chlorophenol pyrolysis investigated by synchrotron radiation photoionization mass spectrometry
    Xu, Ming-Gao
    Huang, Chen
    Zhang, Yi-Fan
    Huang, Jia-Bin
    Zhao, Long
    Lu, Wenchao
    Pan, Yang
    Yang, Jiu-Zhong
    Zhang, Feng
    Cheng, Zhan-Jun
    JOURNAL OF HAZARDOUS MATERIALS, 2024, 480
  • [9] Online Characterization of Isomeric/Isobaric Components in the Gas Phase of Mainstream Cigarette Smoke by Tunable Synchrotron Radiation Vacuum Ultraviolet Photoionization Time-of-Flight Mass Spectrometry and Photoionization Efficiency Curve Simulation
    Pan, Yang
    Hu, Yonghua
    Wang, Jian
    Ye, Lili
    Liu, Chengyuan
    Zhu, Zhixiang
    ANALYTICAL CHEMISTRY, 2013, 85 (24) : 11993 - 12001
  • [10] Measurements of Secondary Organic Aerosol Formed from OH-initiated Photo-oxidation of Isoprene Using Online Photoionization Aerosol Mass Spectrometry
    Fang, Wenzheng
    Gong, Lei
    Zhang, Qiang
    Cao, Maoqi
    Li, Yuquan
    Sheng, Liusi
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012, 46 (07) : 3898 - 3904
12