Phonon-Mediated Quasiparticle Lifetime Renormalizations in Few-Layer Hexagonal Boron Nitride

被引:4
|
作者
Rost, Hakon, I [3 ,8 ]
Cooil, Simon P. [1 ,2 ]
Asland, Anna Cecilie [3 ]
Hu, Jinbang [3 ]
Ali, Ayaz [4 ,5 ]
Taniguchi, Takashi [6 ]
Watanabe, Kenji [7 ]
Belle, Branson D. [4 ]
Holst, Bodil [8 ]
Sadowski, Jerzy T. [9 ]
Mazzola, Federico [10 ,11 ]
Wells, Justin W. [1 ,2 ,3 ]
机构
[1] Univ Oslo UiO, Dept Phys, N-0318 Oslo, Norway
[2] Univ Oslo UiO, Ctr Mat Sci & Nanotechnol, N-0318 Oslo, Norway
[3] Norwegian Univ Sci & Technol NTNU, Dept Phys, N-7491 Trondheim, Norway
[4] SINTEF DIGITAL, Dept Smart Sensor Syst, N-0373 Oslo, Norway
[5] Univ Sindh, Fac Engn & Technol, Dept Elect Engn, Jamshoro 76080, Pakistan
[6] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba 3050044, Japan
[7] Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba 3050044, Japan
[8] Univ Bergen, Dept Phys & Technol, N-5007 Bergen, Norway
[9] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA
[10] Ca Foscari Univ Venice, Dept Mol Sci & Nanosyst, I-30172 Venice, Italy
[11] CNR, Ist Officina Mat, I-34149 Trieste, Italy
关键词
hexagonal boron nitride; graphene heterostructures; many-body interactions; electron-phonon coupling; ARPES; BAND-STRUCTURE; ENCAPSULATED GRAPHENE; ELECTRON; PHOTOEMISSION; INSULATORS; SURFACE; ENERGY;
D O I
10.1021/acs.nanolett.3c02086
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Understanding thecollective behavior of the quasiparticles insolid-state systems underpins the field of nonvolatile electronics,including the opportunity to control many-body effects for well-desiredphysical phenomena and their applications. Hexagonal boron nitride(hBN) is a wide-energy-bandgap semiconductor, showing immense potentialas a platform for low-dimensional device heterostructures. It is aninert dielectric used for gated devices, having a negligible orbitalhybridization when placed in contact with other systems. Despite itsinertness, we discover a large electron mass enhancement in few-layerhBN affecting the lifetime of the & pi;-band states. We show thatthe renormalization is phonon-mediated and consistent with both single-and multiple-phonon scattering events. Our findings thus unveil aso-far unknown many-body state in a wide-bandgap insulator, havingimportant implications for devices using hBN as one of their buildingblocks.
引用
收藏
页码:7539 / 7545
页数:7
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