THE IMPACT OF RELATIVE HUMIDITY ON THE RADIATIVE PROPERTY AND RADIATIVE FORCING OF SULFATE AEROSOL

被引:3
|
作者
张立盛
石广玉
机构
[1] LASG Institute of Atmospheric Physics
[2] Beijing 100029
[3] Chinese Academy of Sciences
关键词
relative humidity; radiative property; radiative forcing;
D O I
暂无
中图分类号
X513 [粒状污染物];
学科分类号
摘要
With the data of complex refractive index of sulfate aerosol,the radiative properties of theaerosol under 8 relative humidity conditions are calculated in this paper.By using the concentrationdistribution from two CTM models and LASG GOALS/AGCM,the radiative forcing due tohygroscopic sulfate aerosol is simulated.The results show that:(1)With the increase of relativehumidity,the mass extinction coefficiency factor decreases in the shortwave spectrum;singlescattering albedo keeps unchanged except for a little increase in longwave spectrum,andasymmetry factor increases in whole spectrum.(2)Larger differences occur in radiative forcingsimulated by using two CTM data,and the global mean forcing is—0.268 and—0.816 W/m~2,respectively.(3)When the impact of relative humidity on radiative property is taken into account,the distribution pattern of radiative forcing due to the wet particles is very similar to that of drysulfate,but the forcing value decreases by 60%.
引用
收藏
页码:465 / 476
页数:12
相关论文
共 50 条
  • [1] Influence of relative humidity on aerosol radiative forcing: An ACE-Asia experiment perspective
    Markowicz, KM
    Flatau, PJ
    Quinn, PK
    Carrico, CM
    Flatau, MK
    Vogelmann, AM
    Bates, D
    Liu, M
    Rood, MJ
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
  • [2] Influences of relative humidity on aerosol optical properties and aerosol radiative forcing during ACE-Asia
    Yoon, Soon-Chang
    Kim, Jiyoung
    ATMOSPHERIC ENVIRONMENT, 2006, 40 (23) : 4328 - 4338
  • [3] Sulfate Aerosol in the Arctic: Source Attribution and Radiative Forcing
    Yang, Yang
    Wang, Hailong
    Smith, Steven J.
    Easter, Richard C.
    Rasch, Philip J.
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2018, 123 (03) : 1899 - 1918
  • [4] Influence of atmospheric relative humidity on ultraviolet flux and aerosol direct radiative forcing: Observation and simulation
    Xia, Dong
    Chen, Ling
    Chen, Huizhong
    Luo, Xuyu
    Deng, Tao
    ASIA-PACIFIC JOURNAL OF ATMOSPHERIC SCIENCES, 2016, 52 (04) : 341 - 352
  • [5] Influence of atmospheric relative humidity on ultraviolet flux and aerosol direct radiative forcing: Observation and simulation
    Dong Xia
    Ling Chen
    Huizhong Chen
    Xuyu Luo
    Tao Deng
    Asia-Pacific Journal of Atmospheric Sciences, 2016, 52 : 341 - 352
  • [6] A physically based estimate of radiative forcing by anthropogenic sulfate aerosol
    Ghan, SJ
    Easter, RC
    Chapman, EG
    Abdul-Razzak, H
    Zhang, Y
    Leung, LR
    Laulainen, NS
    Saylor, RD
    Zaveri, RA
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D6): : 5279 - 5293
  • [7] Numerical study of aerosol radiative forcing over East Asia and the impacts of cloud coverage and relative humidity
    Guo, Jun
    Yin, Yan
    Xu, Meng
    Wu, Jian
    Liu, Duanyang
    Fan, Wenxuan
    Lu, Peng
    ATMOSPHERIC RESEARCH, 2022, 273
  • [8] The impact of molecular interactions on atmospheric aerosol radiative forcing
    Kathmann, Shawn M.
    Schenter, Gregory K.
    Garrett, Bruce C.
    ADVANCES IN QUANTUM CHEMISTRY, VOL 55: APPLICATIONS OF THEORETICAL METHODS TO ATMOSPHERIC SCIENCE, 2008, 55 : 429 - 447
  • [9] Aerosol absorption and radiative forcing
    Stier, P.
    Seinfeld, J. H.
    Kinne, S.
    Boucher, O.
    ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (19) : 5237 - 5261
  • [10] Sensitivity of aerosol optical thickness and aerosol direct radiative effect to relative humidity
    Bian, H.
    Chin, M.
    Rodriguez, J. M.
    Yu, H.
    Penner, J. E.
    Strahan, S.
    ATMOSPHERIC CHEMISTRY AND PHYSICS, 2009, 9 (07) : 2375 - 2386