Negative Ion Conversion by Neutral Carbon Atoms Grazing Scattering from the KI(100) Surface

被引:0
|
作者
Wang, Yiqing [1 ]
Zhou, Hu [1 ]
Wang, He [1 ]
Li, Yuan [3 ]
Feng, Dong [3 ]
Chang, Kaiwen [3 ]
Cong, Yudi [3 ]
Liu, Zhengqi [3 ]
Tu, Zheyan [1 ]
Song, Lixun [1 ]
Wu, Gang [1 ]
Du, Yali [1 ]
Li, Zebin [1 ]
Wu, Qiang [4 ]
Zhang, Xin [6 ]
Zong, Zewen [6 ]
Liu, Yu [3 ]
Zhao, Yongtao [7 ]
Zhang, Hongfei [5 ]
Wang, Guangyi [2 ]
Chen, Ximeng [6 ]
机构
[1] Xian Polytech Univ, Sch Sci, Xian 710600, Peoples R China
[2] Lanzhou City Univ, Sch Elect & Informat Engn, Lanzhou 730000, Peoples R China
[3] Shaanxi Qinzhou Nucl & Radiat Safety Technol Co Lt, Xian 710054, Peoples R China
[4] Lanzhou Univ, Hosp 2, Lanzhou 730000, Peoples R China
[5] Xi An Jiao Tong Univ, Sch Phys, Xian 710049, Peoples R China
[6] Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Peoples R China
[7] Xi An Jiao Tong Univ, Sch Phys, MOE Key Lab Nonequilibrium Synth & Modulat Condens, Xian 710049, Peoples R China
基金
中国国家自然科学基金;
关键词
NANOPARTICLE FORMATION; ELECTRON-CAPTURE; CHARGE-TRANSFER; IMPLANTATION; THRESHOLD; EMISSION; HALIDES; OXYGEN; FRONT; FILMS;
D O I
10.1021/acs.jctc.4c01719
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this work, we performed a theoretical calculation of the negative ion conversion by a neutral carbon atom beam grazing scattering from the KI(100) surface. The Madelung potential, image potential, and ML-polarization interaction contributions are included in the calculation of the electron capture energy defect of the valence band near surface anion sites along the projectile incidence direction. The loss of the formed negative ions does not originate from the electron loss to the unoccupied conduction band or neutral exciton states but results from the Coulomb barrier tunneling detachment of the loosely bound affinity electron to the vacuum level during the interaction with surface lattice anion sites. Here, the large fraction of negative-ion conversion (>= 50%) within the projectile energy range of E p is an element of [5.7,14.9] keV implies the present collision system could be directly used to design the next-generation negative carbon ion sources for the study of isotope shifts in electron affinity, electron correlation effects and for the promotion of nerve tissue repair and regeneration by negative carbon ion irradiation.
引用
收藏
页码:2012 / 2020
页数:9
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