Attosecond impulsive stimulated X-ray Raman scattering in liquid water

被引：1

作者：

Alexander, Oliver ^{[1
]}

Egun, Felix ^{[1
]}

Rego, Laura ^{[1
,2
,3
]}

Gutierrez, Ana Martinez ^{[3
]}

Garratt, Douglas ^{[4
,5
]}

Cardenes, Gustavo Adolfo ^{[3
]}

Nogueira, Juan J. ^{[3
,6
]}

Lee, Jacob P. ^{[1
]}

Zhao, Kaixiang ^{[1
]}

Wang, Ru-Pan ^{[7
]}

Ayuso, David ^{[1
,8
]}

Barnard, Jonathan C. T. ^{[1
]}

Beauvarlet, Sandra ^{[4
,9
]}

Bucksbaum, Philip H. ^{[5
,10
,11
]}

Cesar, David ^{[4
]}

Coffee, Ryan ^{[4
,5
]}

Duris, Joseph ^{[4
]}

Frasinski, Leszek J. ^{[1
]}

Huse, Nils ^{[7
]}

Kowalczyk, Katarzyna M. ^{[1
]}

Larsen, Kirk A. ^{[4
,5
]}

Matthews, Mary ^{[1
]}

Mukamel, Shaul ^{[12
,13
]}

O'Neal, Jordan T. ^{[4
,5
]}

Penfold, Thomas ^{[14
]}

Thierstein, Emily ^{[4
,5
]}

Tisch, John W. G. ^{[1
]}

Turner, James R. ^{[1
]}

Vogwell, Josh ^{[1
]}

Driver, Taran ^{[4
,5
]}

Berrah, Nora ^{[9
]}

Lin, Ming-Fu ^{[4
]}

Dakovski, Georgi L. ^{[4
]}

Moeller, Stefan P. ^{[4
]}

Cryan, James P. ^{[4
,5
]}

Marinelli, Agostino ^{[4
,5
]}

Picon, Antonio ^{[3
,15
]}

Marangos, Jonathan P. ^{[1
]}

机构：

[1] Imperial Coll London, Dept Phys, Blackett Lab, London SW7 2AZ, England

[2] Inst Madrileno Estudios Avanzados Nanociencia iMde, Canto Blanco 28049, Madrid, Spain

[3] Univ Autonoma Madrid, Dept Quim, Madrid 28049, Spain

[4] SLAC Natl Accelerator Lab, Menlo Pk, CA USA

[5] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA USA

[6] Univ Autonoma Madrid, Inst Adv Res Chem Sci IAdChem, Madrid 28049, Spain

[7] Univ Hamburg, Ctr Free Electron Laser Sci, Dept Phys, Luruper Chaussee 149, D-22761 Hamburg, Germany

[8] Max Born Inst, Max Born Str 2A, D-12489 Berlin, Germany

[9] Univ Connecticut, Phys Dept, Storrs, CT 06268 USA

[10] Stanford Univ, Dept Appl Phys, Stanford, CA USA

[11] Stanford Univ, Dept Phys, Stanford, CA USA

[12] Univ Calif Irvine, Dept Chem Phys & Astron, Irvine, CA 92697 USA

[13] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA

[14] Newcastle Univ, Sch Nat & Environm Sci, Chem, Newcastle Upon Tyne NE1 7RU, England

[15] Univ Autonoma Madrid, Condensed Matter Phys Ctr IFIMAC, Madrid 28049, Spain

来源：

SCIENCE ADVANCES | 2024年 / 10卷 / 39期

基金：

英国工程与自然科学研究理事会;

关键词：

MOLECULAR-DYNAMICS SIMULATIONS; 2ND-ORDER PERTURBATION-THEORY; ELASTIC BAND METHOD; SPECTROSCOPY; AMBER;

D O I：

10.1126/sciadv.adp0841

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

We report the measurement of impulsive stimulated x-ray Raman scattering in neutral liquid water. An attosecond pulse drives the excitations of an electronic wavepacket in water molecules. The process comprises two steps: a transition to core-excited states near the oxygen atoms accompanied by transition to valence-excited states. Thus, the wavepacket is impulsively created at a specific atomic site within a few hundred attoseconds through a nonlinear interaction between the water and the x-ray pulse. We observe this nonlinear signature in an intensity-dependent Stokes Raman sideband at 526 eV. Our measurements are supported by our state-of-the-art calculations based on the polarization response of water dimers in bulk solvation and propagation of attosecond x-ray pulses at liquid density.

引用

页数：8

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