Real-space perspective on dephasing in solid-state high harmonic generation

被引:1
|
作者
Brown, Graham G. [1 ]
Jimenez-Galan, Alvaro [1 ,2 ]
Silva, F. [1 ,3 ]
Ivanov, Misha [1 ,4 ,5 ]
机构
[1] Max Born Inst, Max Born Str 2A, D-12489 Berlin, Germany
[2] Natl Res Council Canada, Joint Attosecond Sci Lab, 100 Sussex Dr, Ottawa, ON K1A 0R6, Canada
[3] ICMM, Ctr Super Invest Cient, Sor Juana Ines Cruz,3 Cantoblanco, Madrid 28049, Spain
[4] Humboldt Univ, Dept Phys, Newtonstr 15, D-12489 Berlin, Germany
[5] Imperial Coll London, Blackett Lab, London SW7 2AZ, England
来源
PHYSICAL REVIEW RESEARCH | 2024年 / 6卷 / 04期
关键词
ORDER;
D O I
10.1103/PhysRevResearch.6.043005
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We develop and demonstrate a fully real-space perspective on high harmonic generation (HHG) in crystals. Due to the Wannier-Stark localization induced on subcycle timescales in the presence of a strong field, real-space descriptions are natural for strongly driven solids. Our approach allows us to address the origin of the extremely short dephasing times, which appear necessary for agreement between experimental HHG measurements and theoretical calculations generally performed in reciprocal space. We develop a physically transparent model of real-space dephasing which relates its rate to the distance between different sites in a laser-driven lattice. Our approach leads to well-structured high harmonic spectra at the microscopic level, reproduces the results of macroscopic propagation, and demonstrates that the requirement for ultrafast dephasing times stems from the need for suppressing recombination events with large electron-hole separations during radiative recombination.
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页数:6
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