The third-order nonlinear optical susceptibility in octupolar molecule and its dipolar subunit

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Derkowska, B.
Sahraoui, B.
Nguyen, Phu, X.
Andraud, C.
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| 2001年 / Polish Academy of Sciences卷 / 99期
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The third-order nonlinear optical susceptibility χ [Left Angle Bracket] 3 [Right Angle Bracket] of octupolar molecule with three double bonds was measured using degenerate four wave mixing technique at 532 nm in tetrahydrofuran solution. For comparison, we also measured its analogous dipolar subunit. We found that the χ [Left Angle Bracket] 3 [Right Angle Bracket] value for octupolar molecule is about twice larger than its dipolar subunit.
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