Advanced nitrate removal in sulfur autotrophic denitrification biofilter under dissolved oxygen shock and low temperature enhanced by boron oxide and magnesium oxide: Hydrogen sulfide accumulation and regulation

被引:0
|
作者
Jia, Qingliang [1 ]
Li, Shiwen [2 ]
Meng, Fangang [3 ]
Zhang, Jian [1 ]
Wang, Shengyuan [2 ]
Su, Mengran [1 ]
Jiang, Hao [1 ]
机构
[1] Shandong Univ Sci & Technol, Inst Yellow River Delta Earth Surface Proc & Ecol, Coll Safety & Environm Engn, Qingdao, Peoples R China
[2] Qingdao West Coast Publ Util Grp Water Co Ltd, Qingdao, Peoples R China
[3] Sun Yat Sen Univ, Guangdong Prov Key Lab Environm Pollut Control & R, Guangzhou, Peoples R China
关键词
Sulfur autotrophic denitrification; Boron and magnesium; Seasonal temperature; H2S management; Air-water backwash;
D O I
10.1016/j.jenvman.2024.123268
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Strengthening nitrate removal stability of sulfur autotrophic denitrification (SAD) under environmental stress is of great urgency. This study established a biofilter filled with S0-based filter material modified by boron oxide and magnesium oxide (FMSBMg). Hydrogen sulfide (H2S) accumulation reached 18.89 +/- 4.51 mg/L and 7.28 +/- 2.03 mg/L in summer and winter. Air and water backwash flow rates of 3 m3/h and 150 L/h could reduce H2S accumulation to below 0.16 mg/L under dissolved oxygen (DO) of 4.4 +/- 0.1 mg/L 0.4 +/- 0.1 mg/L B 3+ and 15.9 +/- 0.3 mg/L Mg2+ released from FM SBMg enhanced nitrate removal stability under DO shock and temperature drop. NO3--N eff reached 5.2 +/- 2.2 mg/L at 12.1 +/- 0.8 degrees C. Coexistence of NH4+-N and NO2--N provided substrates for in situ enrichment of Anammox bacteria. Thiobacillus, Lysobacter and Brocadia abundances accounted for 53.9%, 2.5% and 1.8% in biofilter, respectively. This study could provide theoretical basis for SAD biofilter application and H2S regulation.
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页数:12
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