Chaotic mixing process of fly ash in acid leaching tank intensified by rigid-flexible impeller

被引:0
|
作者
Xiong X. [1 ]
Liu Z. [1 ]
Gu D. [1 ]
Qiu F. [1 ]
Wang L. [1 ]
Tao C. [1 ]
Wang Y. [2 ]
机构
[1] School of Chemistry and Chemical Engineering, Chongqing University, Chongqing
[2] Department of Chemical Engineering, Tsinghua University, Beijing
来源
Huagong Xuebao/CIESC Journal | 2019年 / 70卷 / 05期
关键词
Chaotic mixing; Coal ash; Largest Lyapunov exponents; Multi-scale entropy; Rigid-flexible impeller;
D O I
10.11949/j.issn.0438-1157.20181179
中图分类号
学科分类号
摘要
In the traditional fly ash aluminizing process, the acid immersion stirring tank adopts a rigid stirring paddle. Due to the limited pumping capacity of rigid impellers, some problems such as settlement of solid particles, deficiently of chaotic, and low efficiency of mixing in this process often occur in solid-liquid mixing processes. Thus, the rigid-flexible impeller was adopted to enhance solid-liquid chaotic mixing behavior in acid leaching process. In a fly ash-water system with a solids concentration of 30%, the chaotic mixing characteristics and energy dissipation were investigated in STRs equipped with rigid-flexible impeller. Torque sensor was employed to collect the torque time series signal. The largest Lyapunov exponents and the multi-scale entropy were compiled and calculated by Matlab to indicate the degree of chaotic mixing based on the torque time series signal. Meanwhile, the power consumption per unit volume was used to characterize the stirred reactor power characteristics. The effects of impeller types, rotation speed, flexible piece width/length, and impeller off-bottom clearance on chaotic mixing behavior were taken into consideration in the solid-liquid mixing processes. The results showed that the rigid-flexible impeller could effectively promote the chaotic mixing and reduce the accumulation of solid particles at the bottom of STRs in the fly ash-water system. Largest Lyapunov exponents of the system reached the maximum value of 0.0645 and multi-scale entropy was bigger than that of other conditions at the rotation speed of 120 r/min, the off-bottom clearance of T/4, the flexible piece length of 1.2H1 and width of D/8. The power consumption increases exponentially with the increase of rotation speed. © All Right Reserved.
引用
收藏
页码:1693 / 1701
页数:8
相关论文
共 30 条
  • [1] Shemi A., Mpana R.N., Ndlovu S., Et al., Alternative techniques for extracting alumina from coal fly ash, Minerals Engineering, 34, pp. 30-37, (2012)
  • [2] Ding J., Ma S., Zheng S., Et al., Study of extracting alumina from high-alumina PC fly ash by a hydro-chemical process, Hydrometallurgy, 161, pp. 58-64, (2016)
  • [3] Cobo M., Galvez A., Conesa J.A., Et al., Characterization of fly ash from a hazardous waste incinerator in Medellin, Colombia, Journal of Hazardous Materials, 168, 2, pp. 1223-1232, (2009)
  • [4] Xu D., Li H., Bao W., Et al., A new process of extracting alumina from high-alumina coal fly ash in NH<sub>4</sub>HSO<sub>4</sub>+H<sub>2</sub>SO<sub>4</sub> mixed solution, Hydrometallurgy, 165, pp. 336-344, (2016)
  • [5] Nayak N., Panda C.R., Aluminium extraction and leaching characteristics of Talcher thermal power station fly ash with sulphuric acid, Fuel, 89, 1, pp. 53-58, (2010)
  • [6] Doucet F.J., Mohamed S., Neyt N., Et al., Thermochemical processing of a South African ultrafine coal fly ash using ammonium sulphate as extracting agent for aluminium extraction, Hydrometallurgy, 166, pp. 174-184, (2016)
  • [7] Klenov O.P., Noskov A.S., Solid dispersion in the slurry reactor with multiple impellers, Chemical Engineering Journal, 176-177, pp. 75-82, (2011)
  • [8] Bulnes Abundis D., Alvarez M.M., The simplest stirred tank for laminar mixing: mixing in a vessel agitated by an off-centered angled disc, AIChE Journal, 59, 8, pp. 3092-3108, (2013)
  • [9] Nie A., Gao Z., Xue L., Et al., Micromixing performance and the modeling of a confined impinging jet reactor/high speed disperser, Chemical Engineering Science, 184, pp. 14-24, (2018)
  • [10] Liu Z.H., Tang Q., Wang Y.D., Et al., Enhancement of macro-instability in mixer-settler with rigid-flexible impeller, CIESC Journal, 65, 1, pp. 78-86, (2014)