Riser Reactor with a Multistage Oxygen Feeding Strategy for the Oxidative Coupling of Methane

被引：0
|
作者：
Cai M. [1 ]
Chang M. [1 ]
Liu M. [1 ]
Lu C. [1 ]
机构：
[1] State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing
来源：
Industrial and Engineering Chemistry Research | 2024年 / 63卷 / 17期
基金：
中国国家自然科学基金;
关键词：
D O I：
10.1021/acs.iecr.4c00174
中图分类号：
学科分类号：
摘要：
Oxidative coupling of methane (OCM) is characterized by a high temperature and a strongly exothermic reaction. However, the desired C2H4 may easily react to unwanted oxidation products. Due to vigorous gas-solids contacting, excellent heat and mass transfer characteristics, and low gas back-mixing, the riser reactor is adopted in the OCM process. Hydrodynamics and reactor performance of the riser are investigated by simulation. In the riser reactor, the excellent hydrodynamics results in a decrease in consecutive reactions and the heat is released. The multistage oxygen feeding strategy is proposed to improve reactor performance. Compared with the single-stage oxygen feeding, the C2 yield increases by 9.5% in the three-stage oxygen feeding. Moreover, the optimal position of oxygen feeding is presented. © 2024 American Chemical Society
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收藏
页码：7876 / 7890
页数：14
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