Utilization of photocatalytic degradation and efficiency of engineered geopolymer composite tile doped with nano-particles under ultraviolet light

被引:4
|
作者
Shumuye, Eskinder Desta [1 ,4 ]
Liu, Chenxi [2 ]
Fang, Guohao [1 ,3 ]
Mehrpay, Saeid [2 ]
机构
[1] Shenzhen Univ, Inst Adv Study, Shenzhen 518060, Peoples R China
[2] Shenzhen Univ, Sch Civil Engn, Guangdong Prov Key Lab Durabil Marine Civil Engn, Key Lab Durabil Civil Engn Shenzhen, Shenzhen 518060, Peoples R China
[3] Shenzhen Univ, Inst Carbon Neutral, Shenzhen 518060, Peoples R China
[4] Hawassa Univ, Inst Technol, Dept Construct Technol & Management, Hawassa, Ethiopia
来源
基金
中国国家自然科学基金;
关键词
EGC; Self-cleaning; Zinc oxide nanoparticles; LCA; Setting time; Composite; HIGH-PERFORMANCE CONCRETE; ZINC-OXIDE NANOPARTICLES; RHODAMINE-B; MECHANICAL-PROPERTIES; FLY-ASH; CEMENT; HYDRATION; TIO2; WORKABILITY; NANO-SIO2;
D O I
10.1016/j.cemconcomp.2024.105729
中图分类号
TU [建筑科学];
学科分类号
0813 ;
摘要
This study investigates the impact of nano-zinc oxide (ZnO) on the self-cleaning and microstructural performance of engineered geopolymer composites (EGC) for urban cleanliness enhancement. The research focuses on achieving homogeneous dispersion of nano-ZnO through ultrasonication to prevent agglomeration and assess its effects on workability, setting time, mechanical, and microstructural properties of EGC. Results show that incorporating ZnO nanoparticles at 5 % and 10 % concentrations as a surface coating on engineered geopolymer composite creates a highly effective photocatalytic material. This enhanced composite demonstrates significant capability in degrading Rhodamine B (RhB) under UV light exposure over a 15-day period, breaking down organic pollutants into simpler, potentially less toxic substances. The efficiency of degradation depends on factors such as nano-ZnO concentration, UV radiation intensity, and initial pollutant concentration. The optimal dosage of nano-ZnO in EGC is found to be 0.5 %, which enhances hydration and pozzolanic activity, promoting a densified microstructure at the nanoscale. This innovative composite material shows promise as a self-cleaning finishing material for urban buildings, offering potential improvements in both aesthetics and environmental sustainability.
引用
收藏
页数:18
相关论文
共 50 条
  • [1] Photocatalytic degradation of unsymmetrical dimethylhydrazine with Nd-doped ZnO nano-particles
    School of Science, Beijing Institute of Technology, Beijing 100081, China
    不详
    不详
    Beijing Ligong Daxue Xuebao, 2009, 3 (266-269):
  • [2] Physical characterizations of nano-particles α-MoO3: Eosin degradation under visible light
    Koriche, Nesrine
    Brahimi, Razika
    Trari, Mohamed
    REACTION KINETICS MECHANISMS AND CATALYSIS, 2025,
  • [3] Photocatalytic degradation of reactive brilliant blue X-BR with Al-doped ZnO nano-particles
    School of Chemical Engineering and Environment, Beijing Institute of Technology, Beijing 100081, China
    不详
    Guocheng Gongcheng Xuebao, 2008, 1 (54-59):
  • [4] Role of a-Fe2O3 nano-particles in protecting wood from ultraviolet light degradation
    Yi, Tengfei
    Morrell, Jeffrey J.
    HOLZFORSCHUNG, 2023, 77 (06) : 453 - 467
  • [5] A new simple synthesis of CdS nano-particles by composite-molten-salt method and their high photocatalytic degradation activity
    Xiang, Donghu
    Zhu, Yabo
    Cai, Cunjin
    He, Zhanjun
    Liu, Zhangsheng
    Yin, Dagen
    Luo, Jin
    PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2011, 44 (03): : 733 - 737
  • [6] Photocatalytic Degradation of Deoxynivalenol Using Cerium Doped Titanium Dioxide under Ultraviolet Light Irradiation
    He, Pengzhen
    Zhao, Zhiyong
    Tan, Yanglan
    Hengchao, E.
    Zuo, Minghui
    Wang, Jianhua
    Yang, Junhua
    Cui, Shuxin
    Yang, Xianli
    TOXINS, 2021, 13 (07)
  • [7] New carbon quantum dots nano-particles decorated zinc peroxide (Cdots/ZnO2) nano-composite with superior photocatalytic efficiency for removal of different dyes under UV-A light
    El-Shamy, Ahmed Gamal
    SYNTHETIC METALS, 2020, 267
  • [8] Enhanced Photocatalytic Degradation of 4-chlorophenol using Lanthanum Oxide Nano-particles under UVC/Vis Irradiation
    Ghaedrahmat, Zeinab
    Moussavi, Seyedeh Maryam
    Jorfi, Sahand
    Mohasel, Mehrnoosh Abtahi
    Jaafarzadeh, Neamat
    JOURNAL OF NANOSTRUCTURES, 2021, 11 (01) : 165 - 180
  • [9] Pure and Mg-doped self-assembled ZnO nano-particles for the enhanced photocatalytic degradation of 4-chlorophenol
    Selvam, N. Clament Sagaya
    Narayanan, S.
    Kennedy, L. John
    Vijaya, J. Judith
    JOURNAL OF ENVIRONMENTAL SCIENCES, 2013, 25 (10) : 2157 - 2167
  • [10] Pure and Mg-doped self-assembled ZnO nano-particles for the enhanced photocatalytic degradation of 4-chlorophenol
    N.Clament Sagaya Selvam
    S.Narayanan
    L.John Kennedy
    J.Judith Vijaya
    Journal of Environmental Sciences, 2013, (10) : 2157 - 2167