Preparation of S-C3N4/AgCdS Z-Scheme Heterojunction Photocatalyst and Its Effectively Improved Photocatalytic Performance

被引:3
|
作者
Lin, Yuhong [1 ,2 ,3 ]
Chen, Zhuoyuan [1 ,2 ,3 ]
Feng, Chang [1 ,3 ]
Ma, Li [2 ]
Jing, Jiangping [1 ,3 ]
Hou, Jian [2 ]
Xu, Likun [2 ]
Sun, Mingxian [2 ]
Chen, Dongchu [1 ,3 ]
机构
[1] Foshan Univ, Sch Mat Sci & Hydrogen Energy, 18 Jiangwanyi Rd, Foshan 528000, Peoples R China
[2] Luoyang Ship Mat Res Inst LSMRI, State Key Lab Marine Corros & Protect, Wenhai Rd, Qingdao 266237, Peoples R China
[3] Guangdong Key Lab Hydrogen Energy Technol, 18 Jiangwanyi Rd, Foshan 528000, Peoples R China
来源
MOLECULES | 2024年 / 29卷 / 09期
基金
中国国家自然科学基金;
关键词
semiconductor photocatalysis; Z-scheme heterojunction; S-doped graphitic carbon nitride; Ag-doped CdS nanoparticles; photocatalytic degradation; HYDROGEN EVOLUTION; DEGRADATION; CDS;
D O I
10.3390/molecules29091931
中图分类号
Q5 [生物化学]; Q7 [分子生物学];
学科分类号
071010 ; 081704 ;
摘要
In this study, S-doped graphitic carbon nitride (S-C3N4) was prepared using the high-temperature polymerization method, and then S-C3N4/AgCdS heterojunction photocatalyst was obtained using the chemical deposition method through loading Ag-doped CdS nanoparticles (AgCdS NPs) on the surface of S-C3N4. Experimental results show that the AgCdS NPs were evenly dispersed on the surface of S-C3N4, indicating that a good heterojunction structure was formed. Compared to S-C3N4, CdS, AgCdS and S-C3N4/CdS, the photocatalytic performance of S-C3N4/AgCdS has been significantly improved, and exhibits excellent photocatalytic degradation performance of Rhodamine B and methyl orange. The doping of Ag in collaboration with the construction of a Z-scheme heterojunction system promoted the effective separation and transport of the photogenerated carriers in S-C3N4/AgCdS, significantly accelerated its photocatalytic reaction process, and thus improved its photocatalytic performance.
引用
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页数:13
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