Graphitic carbon nitride as an efficient metal-free photocatalyst for tetracycline removal

被引:2
|
作者
da Silva Junior, Afonso Henrique [1 ]
de Oliveira, Carlos Rafael Silva [2 ]
Francisco, Isadora Bertini Martins [2 ]
de Oliveira, Patricia Viera [3 ]
de Aguiar, Catia Rosana Lange [2 ]
da Silva, Adriano [1 ]
机构
[1] Univ Fed Santa Catarina, Dept Chem Engn & Food Engn, Lab Mass Transfer & Numer Simulat Chem Syst, Florianopolis, SC, Brazil
[2] Univ Fed Santa Catarina, Dept Text Engn, Blumenau, SC, Brazil
[3] Univ Fed Santa Catarina, Dept Chem Engn & Food Engn, Florianopolis, SC, Brazil
关键词
Wastewater; antibiotics; photocatalysis; metal-free catalyst; experimental design; DEGRADATION; FABRICATION; G-C3N4;
D O I
10.1142/S1793604724510147
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Tetracycline (TC) is a drug commonly detected in wastewater. Given this, researchers have been working intensely to create efficient methods to eliminate TC from water. Therefore, the work aimed to synthesize a metal-free catalyst, graphitic carbon nitride (g-CN), to remove TC from water through photocatalysis. The one-step methodology via thermal condensation successfully synthesized the catalyst. Also, a Box-Behnken experimental design was used in the TC treatment to optimize variables such as pollutant and catalyst concentration and pH. Under optimized conditions, there was a 79% removal in 2 h. Furthermore, the catalyst was reused in four consecutive cycles, demonstrating remarkable recyclability. Therefore, the catalyst produced proved effective and promising for the aqueous remediation of TC.
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页数:8
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