THEORY OF ULTRAFAST TIME-RESOLVED ABSORPTION-SPECTROSCOPY

被引：2
|
作者：
YEH, CY [1 ]
CHANG, WL [1 ]
MA, H [1 ]
LIN, SH [1 ]
机构：
[1] ARIZONA STATE UNIV,CTR STUDY EARLY EVENTS PHOTOSYNTH,TEMPE,AZ 85287
来源：
INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY | 1991年 / 39卷 / 03期
关键词：
D O I：
10.1002/qua.560390313
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
In this paper, the density matrix formalism has been applied to treat ultrafast time-resolved absorption spectroscopy. We have shown that in the femto-second (fs) pump-probe experiments, the observed time-resolved absorption spectra consist of the contributions from the population (i.e., incoherent contribution) and the coherence (i.e., the phase of the system). The adiabatic approximation has been used to derive the expressions for ultrafast time-resolved spectra. We have also shown that the dynamics of the coherence will result in quantum beat. Numerical calculations have been performed to demonstrate the theoretical results.
引用
收藏
页码：353 / 370
页数：18
相关论文
共 50 条
  • [1] TIME-RESOLVED ABSORPTION-SPECTROSCOPY OF HEMATOPORPHYRIN AND ITS PHOTOPRODUCTS
    ROTOMSKIS, R
    VAICAITIS, V
    PISKARSKAS, A
    CHEMICAL PHYSICS LETTERS, 1993, 202 (3-4) : 233 - 236
  • [2] INTENSE SQUARE FLASH SOURCE FOR TIME-RESOLVED ABSORPTION-SPECTROSCOPY
    PAUR, RJ
    DORSETT, JL
    BAIR, EJ
    REVIEW OF SCIENTIFIC INSTRUMENTS, 1982, 53 (03): : 306 - 307
  • [3] SPIROOXAZINE PHOTOCHROMISM - PICOSECOND TIME-RESOLVED RAMAN AND ABSORPTION-SPECTROSCOPY
    ARAMAKI, S
    ATKINSON, GH
    CHEMICAL PHYSICS LETTERS, 1990, 170 (2-3) : 181 - 186
  • [4] TIME-RESOLVED FLUORESCENCE AND ABSORPTION-SPECTROSCOPY OF PHOTOSYSTEM-I
    HASTINGS, G
    KLEINHERENBRINK, FAM
    LIN, S
    BLANKENSHIP, RE
    BIOCHEMISTRY, 1994, 33 (11) : 3185 - 3192
  • [5] THEORY AND APPLICATION OF TIME-RESOLVED ABSORPTION SPECTROSCOPY
    FUJIMURA, Y
    SCHRODER, H
    LIN, SH
    SCHLAG, EW
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1979, (APR): : 51 - 51
  • [6] Ultrafast time-resolved absorption spectroscopy of geometric isomers of xanthophylls
    Niedzwiedzki, Dariusz M.
    Enriquez, Miriam M.
    LaFountain, Amy M.
    Frank, Harry A.
    CHEMICAL PHYSICS, 2010, 373 (1-2) : 80 - 89
  • [7] Ultrafast time-resolved absorption spectroscopy of geometric isomers of carotenoids
    Niedzwiedzki, Dariusz M.
    Sandberg, Daniel J.
    Cong, Hong
    Sandberg, Megan N.
    Gibson, George N.
    Birge, Robert R.
    Frank, Harry A.
    CHEMICAL PHYSICS, 2009, 357 (1-3) : 4 - 16
  • [8] TIME-RESOLVED PICOSECOND ABSORPTION-SPECTROSCOPY OF THE LAYERED COMPOUND GALLIUM SELENIDE
    YAO, SS
    BUCHERT, J
    ALFANO, RR
    PHYSICAL REVIEW B, 1982, 25 (10): : 6534 - 6537
  • [9] TIME-RESOLVED INDUCED ABSORPTION-SPECTROSCOPY OF A-AS2SE3
    ORENSTEIN, J
    KASTNER, M
    BULLETIN OF THE AMERICAN PHYSICAL SOCIETY, 1980, 25 (03): : 384 - 385
  • [10] Ultrafast Quantum Time-Resolved Spectroscopy
    Kalashnikov, Dmitry A.
    Melik-Gaykazyan, Elizaveta V.
    Kalachev, Alexey A.
    Yu, Ye Feng
    Kuznetsov, Arseniy I.
    Krivitsky, Leonid A.
    2017 CONFERENCE ON LASERS AND ELECTRO-OPTICS EUROPE & EUROPEAN QUANTUM ELECTRONICS CONFERENCE (CLEO/EUROPE-EQEC), 2017,
12345